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Optimization of sodium hydroxide pretreatment and enzyme loading for efficient hydrolysis of rice straw to improve succinate production by metabolically engineered Escherichia coli KJ122 under simultaneous saccharification and fermentation

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논문

Optimization of sodium hydroxide pretreatment and enzyme loading for efficient hydrolysis of rice straw to improve succinate production by metabolically engineered Escherichia coli KJ122 under simultaneous saccharification and fermentation

학술지

Bioresource technology : biomass, bioenergy, biowastes, conversion technologies, biotransformations, production technologies

저자명

Sawisit, Apichai; Jampatesh, Surawee; Jantama, Sirima Suvarnakuta; Jantama, Kaemwich

초록

<P><B>Abstract</B></P> <P>Rice straw was pretreated with sodium hydroxide (NaOH) before subsequent use for succinate production by <I>Escherichia coli</I> KJ122 under simultaneous saccharification and fermentation (SSF). The NaOH pretreated rice straw was significantly enhanced lignin removal up to 95%. With the optimized enzyme loading of 4% cellulase complex + 0.5% xylanase (endo-glucanase 67 CMC-U/g, &beta;-glucosidase 26 pNG-U/g and xylanase 18 CMC-U/g dry biomass), total sugar conversion reached 91.7 &plusmn; 0.8% (w/w). The physicochemical analysis of NaOH pretreated rice straw indicated dramatical changes in its structure, thereby favoring enzymatic saccharification. In batch SSF, succinate production of 69.8 &plusmn; 0.3 g/L with yield and productivity of 0.84 g/g pretreated rice straw and 0.76 &plusmn; 0.02 g/L/h, respectively, was obtained. Fed-batch SSF significantly improved succinate concentration and productivity to 103.1 &plusmn; 0.4 g/L and 1.37 &plusmn; 0.07 g/L/h with a comparable yield. The results demonstrated a feasibility of sequential saccharification and fermentation of rice straw as a promising process for succinate production in industrial scale.</P> <P><B>Highlights</B></P> <P> <UL> <LI> This report is a pioneer study in fermentative succinate production from rice straw. </LI> <LI> Enzymatic saccharification of NaOH pretreated rice straw achieved 90% sugar yield. </LI> <LI> Succinate at 103 g/L (0.84 g/g pretreated rice straw) was obtained by <I>E. coli</I> KJ122. </LI> <LI> The overall succinate production yield of 0.49 g/g rice straw has been proposed. </LI> <LI> Rice straw is a promising agricultural feedstock for an economic succinate production. </LI> </UL> </P>

발행연도

2018

발행기관

Elsevier

ISSN

0960-8524

260

페이지

pp.348-356

주제어

Rice straw; Succinate; Metabolic engineering; Escherichia coli; Simultaneous saccharification and fermentation

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1 2023-12-11
2 2023-12-11

논문; 2018-07-01

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