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Bioelectrochemical systems for simultaneously production of methane and acetate from carbon dioxide at relatively high rate

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논문

Bioelectrochemical systems for simultaneously production of methane and acetate from carbon dioxide at relatively high rate

학술지

International journal of hydrogen energy

저자명

Jiang, Y.; Su, M.; Zhang, Y.; Zhan, G.; Tao, Y.; Li, D.

초록

This study describes the performance of bioelectrochemical systems, based on electrochemically active mixed culture, capable of reducing CO<SUB>2</SUB> to CH<SUB>4</SUB> and CH<SUB>3</SUB>COOH via direct and/or indirect extracellular electron transfer. The metabolic pathway and end products of this mixed culture were highly dependent on the set cathode potentials. Only CH<SUB>4</SUB> and H<SUB>2</SUB> were produced when the cathode potentials were set in the range from -850 to -950 mV (vs. Ag/AgCl). At potentials more negative than -950 mV, CH<SUB>4</SUB>, H<SUB>2</SUB> and CH<SUB>3</SUB>COOH were simultaneously produced. With a relatively large cathode surface area of 49 cm<SUP>-2</SUP>, CH<SUB>4</SUB> and CH<SUB>3</SUB>COOH were produced at high rates of 129.32 mL d<SUP>-1</SUP> and 94.73 mg d<SUP>-1</SUP>, respectively (at potential of -1150 mV). The highest current capture efficiency reached to 97% in batch potentiostatic experiments. These results presented here suggest that mixed culture show the ability to directly accept electrons from the electrode and abiotically produce H<SUB>2</SUB> to convert CO<SUB>2</SUB> into various organic compounds.

발행연도

2013

발행기관

Pergamon Press ; Elsevier Science Ltd

ISSN

0360-3199

ISSN

1879-3487

38

8

페이지

pp.3497-3502

주제어

Bioelectrochemical systems; Carbon dioxide; Methane; Acetate; Biocathode

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1 2023-12-11
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논문; 2013-03-01

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