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Elimination of formate production in Clostridium thermocellum

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논문

Elimination of formate production in Clostridium thermocellum

학술지

Journal of industrial microbiology & biotechnology

저자명

Rydzak, Thomas; Lynd, Lee R.; Guss, Adam M.

초록

<P>The ability of <I>Clostridium thermocellum</I> to rapidly degrade cellulose and ferment resulting hydrolysis products into ethanol makes it a promising platform organism for cellulosic biofuel production via consolidated bioprocessing. Currently, however, ethanol yield is far below theoretical maximum due to branched product pathways that divert carbon and electrons towards formate, H<SUB>2</SUB>, lactate, acetate, and secreted amino acids. To redirect carbon and electron flux away from formate, genes encoding pyruvate:formate lyase (<I>pflB</I>) and PFL-activating enzyme (<I>pflA</I>) were deleted. Formate production in the resulting &Delta;<I>pfl</I> strain was eliminated and acetate production decreased by 50&nbsp;% on both complex and defined medium. The growth rate of the &Delta;<I>pfl</I> strain decreased by 2.9-fold on defined medium and biphasic growth was observed on complex medium. Supplementation of defined medium with 2&nbsp;mM formate restored &Delta;<I>pfl</I> growth rate to 80&nbsp;% of the parent strain. The role of <I>pfl</I> in metabolic engineering strategies and C<SUB>1</SUB> metabolism is discussed.</P><P><B>Electronic supplementary material</B></P><P>The online version of this article (doi:10.1007/s10295-015-1644-3) contains supplementary material, which is available to authorized users.</P>

발행연도

2015

발행기관

Springer Berlin Heidelberg

ISSN

1367-5435

ISSN

1476-5535

42

9

페이지

pp.1263-1272

주제어

Cellulosic ethanol; Clostridium thermocellum; Pyruvate:formate lyase; Metabolic engineering; C1 metabolism

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1 2023-12-11

논문; 2015-12-31

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