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Metabolic engineering of the marine bacteria Neptunomonas concharum for the production of acetoin and meso-2,3-butanediol from acetate

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논문

Metabolic engineering of the marine bacteria Neptunomonas concharum for the production of acetoin and meso-2,3-butanediol from acetate

학술지

Biochemical engineering journal

저자명

Li, Wei; Pu, Nan; Liu, Chang-Xia; Yuan, Qi-Peng; Li, Zheng-Jun

초록

<P><B>Abstract</B></P> <P>The marine bacteria <I>Neptunomonas concharum</I> was firstly characterized in 2012 and grew optimally at 37 &deg;C, whereas the other species of <I>Neptunomonas</I> showed a lower range of temperature to grow. In this study, we described the achievement of metabolic engineering of <I>N. concharum</I> for the synthesis of acetoin and <I>meso</I>-2,3-butanediol. First, a series of carbon sources were used to cultivate <I>N. concharum</I>. Acetate and succinate were found to be suitable substrates to support effective cell growth. Second, a general electransformation procedure was developed. The optimized transformation efficiency reached about 3 &times; 10<SUP>3</SUP> cfu/&mu;g DNA. Third, the heterologous acetoin and <I>meso</I>-2,3-butanediol biosynthesis pathway was functionally expressed in <I>N. concharum</I>. In shake flask cultivation, the titers of acetoin and <I>meso</I>-2,3-butanediol reached 0.11 g/L. Finally, malic enzyme was overexpressed to improve intracellular pyruvate availability, which significantly improved acetoin and <I>meso</I>-2,3-butanediol titers to 0.56 g/L and 0.38 g/L, respectively. Our results demonstrate that <I>N. concharum</I> has a promising potential to manufacture bulk chemicals using acetate as the carbon source.</P> <P><B>Highlights</B></P> <P> <UL> <LI> The marine bacteria <I>Neptunomonas concharum</I> could efficiently utilize acetate. </LI> <LI> A general electransformation procedure was developed for <I>N. concharum</I>. </LI> <LI> Acetoin and <I>meso</I>-2,3-butanediol biosynthesis pathway was functionally expressed. </LI> <LI> The titers of acetoin and <I>meso</I>-2,3-butanediol reached 0.56 g/L and 0.38 g/L, respectively. </LI> </UL> </P>

발행연도

2019

발행기관

Elsevier

ISSN

1369-703x

151

페이지

pp.107311

주제어

Acetate; Acetoin; 2,3-Butanediol; Metabolic engineering; Neptunomonas concharum

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1 2023-12-11

논문; 2019-11-01

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