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Automatic redirection of carbon flux between glycolysis and pentose phosphate pathway using an oxygen-responsive metabolic switch in Corynebacterium glutamicum

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바이오화학분류
    • 바이오플라스틱
      1. 고무
      2. 플라스틱
    • 바이오정밀화학
      1. 용매
      2. 화학제품
    • 화장품용 기능성소재
      1. 기능성
      2. 계면활성제⁄증점제
    • 의료용 화학소재
      1. 식품첨가제
논문

Automatic redirection of carbon flux between glycolysis and pentose phosphate pathway using an oxygen-responsive metabolic switch in Corynebacterium glutamicum

학술지

ACS Synthetic biology

저자명

Kobayashi, Shunsuke; Kawaguchi, Hideo; Shirai, Tomokazu; Ninomiya, Kazuaki; Takahashi, Kenji; Kondo, Akihiko; Tsuge, Yota

초록

<P>Controlling the carbon flux into a desired pathway is important for improving product yield in metabolic engineering. After entering a cell, glucose is channeled into glycolysis and the pentose phosphate pathway (PPP), which decreases the yield of target products whose synthesis relies on NADPH as a cofactor. Here, we demonstrate redirection of carbon flux into PPP under aerobic conditions in <I>Corynebacterium glutamicum</I>, achieved by replacing the promoter of glucose 6-phosphate isomerase gene (<I>pgi</I>) with an anaerobic-specific promoter of the lactate dehydrogenase gene (<I>ldhA</I>). The promoter replacement increased the split ratio of carbon flux into PPP from 39 to 83% under aerobic conditions. The titer, yield, and production rate of 1,5-diaminopentane, whose synthesis requires NADPH as a cofactor, were increased by 4.6-, 4.4-, and 2.6-fold, respectively. This is the largest improvement in the production of 1,5-diaminopentane or its precursor, lysine, reported to date. After aerobic cell growth, <I>pgi</I> expression was automatically induced under anaerobic conditions, altering the carbon flux from PPP to glycolysis, to produce succinate in a single metabolically engineered strain. Such an automatic redirection of metabolic pathway using an oxygen-responsive switch enables two-stage fermentation for efficient production of two different compounds by a single strain, potentially reducing the production costs and time for practical applications.</P><BR>[FIG OMISSION]</BR>

발행연도

2020

발행기관

American Chemical Society

ISSN

2161-5063

9

4

페이지

pp.814-826

주제어

Corynebacterium glutamicum; glycolysis; pentose phosphate pathway; glucose 6-phosphate isomerase; metabolic switch; oxygen

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논문; 2020-12-31

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