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Ag43-mediated display of a thermostable β-glucosidase in Escherichia coli and its use for simultaneous saccharification and fermentation at high temperatures

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      1. 플라스틱
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논문

Ag43-mediated display of a thermostable β-glucosidase in Escherichia coli and its use for simultaneous saccharification and fermentation at high temperatures

학술지

Microbial cell factories

저자명

Muñ oz-Gutié rrez, Ivá n; Moss-Acosta, Cessna; Trujillo-Martinez, Berenice; Gosset, Guillermo; Martinez, Alfredo

초록

<P><B>Background</B></P><P>The autotransporter (AT) system can potentially be used in the secretion of saccharolytic enzymes for the production of lignocellulosic biofuels and chemicals using <I>Escherichia coli</I>. Although ATs share similar structural characteristics, their capacity for secreting heterologous proteins widely varies. Additionally, the saccharolytic enzyme selected to be secreted should match the cell growth or cell fermentation conditions of <I>E. coli</I>.</P><P><B>Results</B></P><P>In the search for an AT that suits the physiological performance of the homo-ethanologenic <I>E. coli</I> strain MS04, an expression plasmid based on the AT antigen 43 (Ag43) from <I>E. coli</I> was developed. The <I>&beta;</I>-glucosidase BglC from the thermophile bacterium <I>Thermobifida fusca</I> was displayed on the outer membrane of the <I>E. coli</I> strain MS04 using the Ag43 system (MS04/pAg43BglC). This strain was used to hydrolyze and ferment 40&nbsp;g/L of cellobiose in mineral media to produce 16.65&nbsp;g/L of ethanol in 48&nbsp;h at a yield of 81% of the theoretical maximum. Knowing that BglC shows its highest activity at 50°C and retains more than 70% of its activity at pH&nbsp;6, therefore <I>E. coli</I> MS04/pAg43BglC was used to ferment crystalline cellulose (Avicel) in a simultaneous saccharification and fermentation (SSF) process using a commercial cocktail of cellulases (endo and exo) at pH&nbsp;6 and at a relatively high temperature for <I>E. coli</I> (45°C). As much as 22&nbsp;g/L of ethanol was produced in 48&nbsp;h.</P><P><B>Conclusions</B></P><P>The Ag43-BglC system can be used in <I>E. coli</I> strains without commercial <I>&beta;</I>-glucosidases, reducing the quantities of commercial enzymes needed for the SSF process. Furthermore, the present work shows that <I>E. coli</I> cells are able to ferment sugars at 45°C during the SSF process using 40&nbsp;g/L of Avicel, reducing the gap between the working conditions of the commercial saccharolytic enzymes and ethanologenic <I>E. coli</I>.</P>

발행연도

2014

발행기관

BioMed Central

라이선스

cc-by

ISSN

1475-2859

13

페이지

pp.106-106

주제어

Ethanologenic Escherichia coli; Simultaneous saccharification and fermentation; Cellulose; Autotransporter Ag43; Thermobifida fusca β-glucosidase; Ethanol

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1 2023-12-11

논문; 2014-08-01

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