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Multi-modular engineering for renewable production of isoprene via mevalonate pathway in Escherichia coli

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논문

Multi-modular engineering for renewable production of isoprene via mevalonate pathway in Escherichia coli

학술지

Journal of applied microbiology

저자명

Liu, C.‐ L.; Dong, H.‐ G.; Zhan, J.; Liu, X.; Yang, Y.

초록

<P><B>Abstract</B></P><P><B>Aims</B></P><P>To establish the biotechnology platforms for production of bio&#8208;based chemicals in various micro&#8208;organisms is considered as a promising target to improve renewable production of isoprene.</P><P><B>Methods and Results</B></P><P>In this study, we heterologously expressed the mevalonate (MVA) isoprene biosynthesis pathway, and explored three strategies of increasing isoprene production in <I>Escherichia coli</I>. We first manipulated the expression levels of the MVA pathway genes through changing the gene cassettes and promoters. To introduce cofactor engineering, we then overexpressed NADP&#8208;dependent glyceraldehyde&#8208;3&#8208;phosphate dehydrogenase gene from <I>Clostridium acetobutylicum</I> to supply available NADPH. To reduce the inhibitory by&#8208;product accumulation, we finally knocked out acetate&#8208;producing genes, phosphate acetyl transferase and pyruvate oxidase B in <I>E. coli</I>JM109 (DE3), decreasing acetate accumulation 89% and increasing isoprene production 39%. The strategies described here finally increased the isoprene titre to 92 mg l<SUP>&minus;1</SUP> in two&#8208;gene deletion strain JMAB&#8208;4T7P1Trc, increasing 2&middot;6&#8208;fold comparing to strain JM7T7.</P><P><B>Conclusion</B></P><P>The multimodularly engineering approaches including promoter engineering, cofactor engineering and by&#8208;product reducing could be used to improve isoprene production in <I>E. coli</I>.</P><P><B>Significance and Impact of the Study</B></P><P>The metabolic strategies in this study show us directions for further studies to promote transformation of renewable sources to isoprene.</P>

발행연도

2019

ISSN

1364-5072

ISSN

1365-2672

126

4

페이지

pp.1128-1139

주제어

Escherichia coli; gene knockout; isoprene; mevalonate pathway; NADPH regeneration

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논문; 2019-12-31

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