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Redistribution of carbon flux toward 2,3-butanediol production in Klebsiella pneumoniae by metabolic engineering

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논문

Redistribution of carbon flux toward 2,3-butanediol production in Klebsiella pneumoniae by metabolic engineering

학술지

PloS one

저자명

Kim, Borim; Lee, Soojin; Jeong, Daun; Yang, Jeongmo; Oh, Min-Kyu; Lee, Jinwon

초록

<P><I>Klebsiella pneumoniae</I> KCTC2242 has high potential in the production of a high-value chemical, 2,3-butanediol (2,3-BDO). However, accumulation of metabolites such as lactate during cell growth prevent large-scale production of 2,3-BDO. Consequently, we engineered <I>K. pneumoniae</I> to redistribute its carbon flux toward 2,3-BDO production. The <I>ldhA</I> gene deletion and gene overexpression (<I>budA</I> and <I>budB</I>) were conducted to block a pathway that competitively consumes reduced nicotinamide adenine dinucleotide and to redirect carbon flux toward 2,3-BDO biosynthesis, respectively. These steps allowed efficient glucose conversion to 2,3-BDO under slightly acidic conditions (pH 5.5). The engineered strain SGSB105 showed a 40% increase in 2,3-BDO production from glucose compared with that of the host strain, SGSB100. Genes closely related to 2,3-BDO biosynthesis were observed at the gene transcription level by cultivating the SGSB100, SGSB103, SGSB104, and SGSB105 strains under identical growth conditions. Transcription levels for <I>budA</I>, <I>budB</I>, and <I>budC</I> increased approximately 10% during the log phase of cell growth relative to that of SGSB100. Transcription levels of 2,3-BDO genes in SGSB105 remained high during the log and stationary phases. Thus, the carbon flux was redirected toward 2,3-BDO production. Data on batch culture and gene transcription provide insight into improving the metabolic network for 2,3-BDO biosynthesis for industrial applications.</P>

발행연도

2014

발행기관

Public Library of Science

라이선스

cc-by

ISSN

1932-6203

9

10

페이지

pp.e105322

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논문; 2014-10-20

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