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Ionic liquids for the concomitant use in extremophiles lysis and extremozymes extraction

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논문

Ionic liquids for the concomitant use in extremophiles lysis and extremozymes extraction

학술지

Bioresource technology : biomass, bioenergy, biowastes, conversion technologies, biotransformations, production technologies

저자명

Gutié rrez-Arnillas, E.; Deive, F.J.; Sanromá n, M.A.; Rodrí guez, A.

초록

<P><B>Abstract</B></P> <P>Ionic liquids have been successfully proposed to modify membrane permeability in cultures of a model extremophilic bacterium <I>Thermus thermophilus</I> HB27, which makes up the first time that aqueous solutions of these molten salts are applied in downstream stages of this kind of microorganisms. The presence of 1g/L of C<SUB>10</SUB>MIMCl entails a great solubilisation of cell biomass, thus allowing the release of intracellular and membrane-bound enzyme. The influence on the enzyme activity of two inorganic salts such as Na<SUB>2</SUB>CO<SUB>3</SUB> and (NH<SUB>4</SUB>)<SUB>2</SUB>SO<SUB>4</SUB>, selected on the basis of their high salting out potential and biocompatibility with enzymes, respectively, was investigated. In parallel, their ability to trigger phase segregation was confirmed in the presence of the enzyme crude, leading to very high levels of enzyme extraction (96%). The validity of the strategy was confirmed by operating at bioreactor scale, and the main bioprocess parameters were obtained by modelling the experimental data.</P> <P><B>Highlights</B></P> <P> <UL> <LI> C<SUB>10</SUB>MIMCl showed an outstanding lysis ability in cultures of <I>Thermus thermophilus</I> HB27. </LI> <LI> Na<SUB>2</SUB>CO<SUB>3</SUB> and (NH<SUB>4</SUB>)<SUB>2</SUB>SO<SUB>4</SUB> were efficient salting out agents in C<SUB>10</SUB>MIMCl aqueous solutions. </LI> <LI> The combination of (NH<SUB>4</SUB>)<SUB>2</SUB>SO<SUB>4</SUB> and C<SUB>10</SUB>MIMCl allowed extracting 96% of lipolytic enzymes. </LI> </UL> </P> <P><B>Graphical abstract</B></P> <P>[DISPLAY OMISSION]</P>

발행연도

2015

발행기관

Elsevier

ISSN

0960-8524

186

페이지

pp.303-308

주제어

Thermus thermophilus HB27; Extremophiles; Lipolytic enzymes; Ionic liquids; Aqueous biphasic systems

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1 2023-12-11

논문; 2015-06-01

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