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The Weimberg pathway: an alternative for Myceliophthora thermophila to utilize D-xylose

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논문

The Weimberg pathway: an alternative for Myceliophthora thermophila to utilize D-xylose

학술지

Biotechnology for biofuels and bioproducts

저자명

Liu, Defei; Zhang, Yongli; Li, Jingen; Sun, Wenliang; Yao, Yonghong; Tian, Chaoguang

초록

<P><B>Background</B></P><P>With <SMALL>D</SMALL>-xylose being the second most abundant sugar in nature, its conversion into products could significantly improve biomass-based process economy. There are two well-studied phosphorylative pathways for <SMALL>D</SMALL>-xylose metabolism. One is isomerase pathway mainly found in bacteria, and the other one is <I>oxo</I>-reductive pathway that always exists in fungi. Except for these two pathways, there are also non-phosphorylative pathways named xylose oxidative pathways and they have several advantages over traditional phosphorylative pathways. In <I>Myceliophthora thermophila</I>, <SMALL>D</SMALL>-xylose can be metabolized through <I>oxo</I>-reductive pathway after plant biomass degradation. The survey of non-phosphorylative pathways in this filamentous fungus will offer a potential way for carbon-efficient production of fuels and chemicals using <SMALL>D</SMALL>-xylose.</P><P><B>Results</B></P><P>In this study, an alternative for utilization of <SMALL>D</SMALL>-xylose, the non-phosphorylative Weimberg pathway was established in <I>M. thermophila</I>. Growth on <SMALL>D</SMALL>-xylose of strains whose <SMALL>D</SMALL>-xylose reductase gene was disrupted, was restored after overexpression of the entire Weimberg pathway. During the construction, a native <SMALL>D</SMALL>-xylose dehydrogenase with highest activity in <I>M. thermophila</I> was discovered. Here, <I>M. thermophila</I> was also engineered to produce 1,2,4&#x2010;butanetriol using <SMALL>D</SMALL>-xylose through non-phosphorylative pathway. Afterwards, transcriptome analysis revealed that the <SMALL>D</SMALL>-xylose dehydrogenase gene was obviously upregulated after deletion of <SMALL>D</SMALL>-xylose reductase gene when cultured in a <SMALL>D</SMALL>-xylose medium. Besides, genes involved in growth were enriched in strains containing the Weimberg pathway.</P><P><B>Conclusions</B></P><P>The Weimberg pathway was established in <I>M. thermophila</I> to support its growth with <SMALL>D</SMALL>-xylose being the sole carbon source. Besides, <I>M. thermophila</I> was engineered to produce 1,2,4&#x2010;butanetriol using <SMALL>D</SMALL>-xylose through non-phosphorylative pathway. To our knowledge, this is the first report of non-phosphorylative pathway recombinant in filamentous fungi, which shows great potential to convert <SMALL>D</SMALL>-xylose to valuable chemicals.</P><P><B>Supplementary Information</B></P><P>The online version contains supplementary material available at 10.1186/s13068-023-02266-7.</P>

발행연도

2023

발행기관

BioMed Central

ISSN

2731-3654

16

1

페이지

pp.13

주제어

Myceliophthora; D-Xylose; D-Xylose dehydrogenase; Weimberg pathway; 1,2,4&#x2010; Butanetriol;

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논문; 2023-01-23

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