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Functional assembly of a multi-enzyme methanol oxidation cascade on a surface-displayed trifunctional scaffold for enhanced NADH production

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논문

Functional assembly of a multi-enzyme methanol oxidation cascade on a surface-displayed trifunctional scaffold for enhanced NADH production

학술지

Chemical communications : Chem comm

저자명

Liu, Fang; Banta, Scott; Chen, Wilfred

초록

<P>We report a simple and low-cost strategy that allows the sequential and site-specific assembly of a dehydrogenase-based multi-enzyme cascade for methanol oxidation on the yeast surface using the high-affinity interactions between three orthogonal cohesin&ndash;dockerin pairs. The multi-enzyme cascade showed 5 times higher NADH production rate than the non-complexed enzyme mixture, a result of efficient substrate channeling.</P><BR><BR><P>Graphic Abstract</P><P>We report a simple and low-cost strategy that allows the sequential and site-specific assembly of a dehydrogenase-based multi-enzyme cascade for methanol oxidation on the yeast surface with up to 5 times higher NADH production rate than free enzymes.<BR><IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c3cc40454d'><BR></P>

발행연도

2013

발행기관

The Royal Society of Chemistry

ISSN

1359-7345

ISSN

1364-548x

49

36

페이지

pp.3766-3768

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1 2023-12-11

논문; 2013-01-01

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