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Metabolic engineering of Clostridium tyrobutyricum for n-butanol production through co-utilization of glucose and xylose

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논문

Metabolic engineering of Clostridium tyrobutyricum for n-butanol production through co-utilization of glucose and xylose

학술지

Biotechnology and bioengineering

저자명

Yu, Le; Xu, Mengmeng; Tang, I‐ Ching; Yang, Shang‐ Tian

초록

<P><B>ABSTRACT</B></P><P>The glucose&#8208;mediated carbon catabolite repression (CCR) in <I>Clostridium tyrobutyricum</I> impedes efficient utilization of xylose present in lignocellulosic biomass hydrolysates. In order to relieve the CCR and enhance xylose utilization, three genes (<I>xylT</I>, <I>xylA</I>, and <I>xylB</I>) encoding a xylose proton&#8208;symporter, a xylose isomerase and a xylulokinase, respectively, from <I>Clostridium acetobutylicum</I> ATCC 824 were co&#8208;overexpressed with aldehyde/alcohol dehydrogenase (adhE2) in <I>C. tyrobutyricum</I> (&Delta;<I>ack</I>). Compared to the strain Ct(&Delta;<I>ack</I>)&#8208;pM2 expressing only <I>adhE2</I>, the mutant Ct(&Delta;<I>ack</I>)&#8208;pTBA had a higher xylose uptake rate and was able to simultaneously consume glucose and xylose at comparable rates for butanol production. Ct(&Delta;<I>ack</I>)&#8208;pTBA produced more butanol (12.0 vs. 3.2&thinsp;g/L) with a higher butanol yield (0.12 vs. 0.07&thinsp;g/g) and productivity (0.17 vs. 0.07&thinsp;g/L&thinsp;&middot;&thinsp;h) from both glucose and xylose, while Ct(&Delta;<I>ack</I>)&#8208;pM2 consumed little xylose in the fermentation. The results confirmed that the CCR in <I>C. tyrobutyricum</I> could be overcome through overexpressing <I>xylT</I>, <I>xylA</I>, and <I>xylB</I>. The mutant was also able to co&#8208;utilize glucose and xylose present in soybean hull hydrolysate (SHH) for butanol production, achieving a high butanol titer of 15.7&thinsp;g/L, butanol yield of 0.24&thinsp;g/g, and productivity of 0.29&thinsp;g/L&thinsp;&middot;&thinsp;h. This study demonstrated the potential application of Ct(&Delta;<I>ack</I>)&#8208;pTBA for industrial biobutanol production from lignocellulosic biomass. Biotechnol. Bioeng. 2015;112: 2134&ndash;2141. &copy; 2015 Wiley Periodicals, Inc.</P>

발행연도

2015

ISSN

0006-3592

ISSN

1097-0290

112

10

페이지

pp.2134-2141

주제어

butanol; carbon catabolite repression; Clostridium tyrobutyricum; soybean hull hydrolysate; xylose; metabolic engineering

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1 2023-12-11
2 2023-12-11

논문; 2015-12-31

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