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Enzymatic halogenation of the phenolic monoterpenes thymol and carvacrol with chloroperoxidase

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논문

Enzymatic halogenation of the phenolic monoterpenes thymol and carvacrol with chloroperoxidase

학술지

Green chemistry : an international journal and green chemistry resource : GC

저자명

Getrey, Laura; Krieg, Thomas; Hollmann, Frank; Schrader, Jens; Holtmann, Dirk

초록

<P>The conversion of the phenolic monoterpenes thymol and carvacrol into antimicrobials by (electro)-chemoenzymatic halogenation was investigated using a chloroperoxidase (CPO) catalyzed process. The CPO catalysed process enables for the first time the biotechnological production of chlorothymol, chlorocarvacrol and bromothymol as well as a dichlorothymol with high conversion rates, total turnover numbers and space time yields of up to 90%, 164 000 and 4.6 mM h<SUP>&minus;1</SUP>, respectively.</P><BR><BR><P>Graphic Abstract</P><P>Enzymatic halogenation of thymol and its derivatives has been shown using a bioelectrochemical approach with chloroperoxidase.<BR><IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c3gc42269k'><BR></P>

발행연도

2014

발행기관

The Royal Society of Chemistry

ISSN

1463-9262

ISSN

1463-9270

16

3

페이지

pp.1104-1108

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논문; 2014-01-01

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