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Development of an Immobilized Ketoreductase for Enzymatic (R)-1-(3,5-Bis(trifluoromethyl)phenyl)ethanol Production

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논문

Development of an Immobilized Ketoreductase for Enzymatic (R)-1-(3,5-Bis(trifluoromethyl)phenyl)ethanol Production

학술지

Organic process research & development

저자명

Li, Hongmei; Moncecchi, Johannah; Truppo, Matthew D.

초록

<P>The development of an immobilized ketoreductase via covalent binding on resin EC-HFA has demonstrated that it is highly active and stable in organic solvents and can be recycled and reused many times in both batch mode and flow reactor mode. (<I>R</I>)-1-(3,5-Bis(trifluoromethyl)phenyl)ethanol, a key chiral intermediate in the synthesis of EMEND, was synthesized in 98% yield with >99% ee using the immobilized ketoreductase in a 50% hexanes/40% IPA/10% water solvent system. The immobilized ketoreductase has also been applied to the synthesis of various chiral alcohols.</P><P><B>Graphic Abstract</B><BR><IMG SRC='http://pubs.acs.org/appl/literatum/publisher/achs/journals/content/oprdfk/2015/oprdfk.2015.19.issue-7/op5003215/production/images/medium/op-2014-003215_0017.gif'></P>

발행연도

2015

발행기관

American Chemical Society

ISSN

1083-6160

ISSN

1520-586x

19

7

페이지

pp.695-700

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논문; 2015-12-31

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