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Ethanol production from xylose by a recombinant Candida utilis strain expressing protein-engineered xylose reductase and xylitol dehydrogenase

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논문

Ethanol production from xylose by a recombinant Candida utilis strain expressing protein-engineered xylose reductase and xylitol dehydrogenase

학술지

Bioscience, biotechnology, and biochemistry

저자명

TAMAKAWA, Hideyuki; IKUSHIMA, Shigehito; YOSHIDA, Satoshi

초록

<P>The industrial yeast <I>Candida utilis</I> can grow on media containing xylose as sole carbon source, but cannot ferment it to ethanol. The deficiency might be due to the low activity of NADPH-preferring xylose reductase (XR) and NAD<SUP>+</SUP>-dependent xylitol dehydogenase (XDH), which convert xylose to xylulose, because <I>C. utilis</I> can ferment xylulose. We introduced multiple site-directed mutations in the coenzyme binding sites of XR and XDH derived from the xylose-fermenting yeast <I>Candida shehatae</I> to alter their coenzyme specificities. Several combinations of recombinant and native XRs and XDHs were tested. Highest productivity was observed in a strain expressing CsheXR K275R/N277D (NADH-preferring) and native CsheXDH (NAD<SUP>+</SUP>-dependent), which produced 17.4 g/L of ethanol from 50 g/L of xylose in 20 h. Analysis of the genes responsible for ethanol production from the xylose capacity of <I>C. utilis</I> indicated that the introduction of CsheXDH was essential, while overexpression of CsheXR K275R/N277D improved efficiency of ethanol production.</P>

발행연도

2011

발행기관

Japan Society for Bioscience, Biotechnology, and Agrochemistry

ISSN

0916-8451

ISSN

1347-6947

75

10

페이지

pp.1994-2000

주제어

Candida utilis; xylose; ethanol; intracellular NADH/NAD+ concentration

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논문; 2011-12-31

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