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Amino Aldehydes Revisited

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논문

Amino Aldehydes Revisited

학술지

European journal of organic chemistry

저자명

Mestrom, Luuk; Bracco, Paula; Hanefeld, Ulf

초록

<P>The enzymatic oxidation of amino alcohols was studied to address the long&#8208;standing problem of product stability. Amino aldehydes, highly sought and unstable compounds, can be generated under mild conditions if they are immediately protected. Utilizing a range of alcohol dehydrogenases (ADHs) and semicarbazide as a scavenger, the enantioselective synthesis of protected amino aldehydes is possible. Glycerol dehydrogenase from <I>Gluconobacter oxydans</I> (<I>Go</I>GDH) displayed excellent enantioselectivity but limited substrate scope, whereas horse liver ADH catalyzed a broad range of conversions with low enantioselectivities.</P>

발행연도

2017

ISSN

1434-193x

ISSN

1099-0690

47

페이지

pp.7019-7025

주제어

Amino alcohols; Amino aldehydes; Biocatalysis; Enzymes; Oxidation

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논문; 2017-12-18

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