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Structures of L-proline trans-hydroxylase reveal the catalytic specificity and provide deeper insight into AKG-dependent hydroxylation

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논문

Structures of L-proline trans-hydroxylase reveal the catalytic specificity and provide deeper insight into AKG-dependent hydroxylation

학술지

Acta crystallographica. Section D, Structural biology

저자명

Hu, Xiaoyan; Huang, Xue; Liu, Jiao; Zheng, Ping; Gong, Weimin; Yang, Lin

초록

<P>L-Proline hydroxylase is a member of the non-heme Fe<SUP>2+</SUP>/&alpha;-ketoglutarate (AKG)-dependent hydroxylase family that catalyzes the reaction from L-proline to hydroxy-L-proline, which is widely used in drug synthesis, biochemistry, food supplementation and cosmetic industries. Here, the first crystal structure of L-proline <I>trans</I>-hydroxylase and its complexes with substrate and product are reported, which reveal the structural basis of <I>trans-cis</I> proline hydroxylation selectivity. Structure comparison with other AKG-dependent hydroxylases identifies conserved amino acid residues, which may serve as signatures of in-line or off-line AKG binding modes in the AKG-dependent enzyme family.</P>

발행연도

2023

발행기관

International Union of Crystallography

ISSN

0907-4449

ISSN

2059-7983

79

4

페이지

pp.318-325

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1 2023-12-11

논문; 2023-04-01

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