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Continuous-Flow Reactor-Based Enzymatic Synthesis of Phosphorylated Compounds on Large Scale

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논문

Continuous-Flow Reactor-Based Enzymatic Synthesis of Phosphorylated Compounds on Large Scale

학술지

Chemistry : a European journal

저자명

Babich, Lara; Hartog, Aloysius F.; van  der  Horst, Michael A.; Wever, Ron

초록

<P><B>Abstract</B></P><P>Acid phosphatase, an enzyme that is able to catalyze the transfer of a phosphate group from cheap pyrophosphate to alcoholic substrates, was covalently immobilized on polymethacrylate beads with an epoxy linker (Immobeads&#8208;150 or Sepabeads EC&#8208;EP). After immobilization 70&thinsp;% of the activity was retained and the immobilized enzyme was stable for many months. With the immobilized enzyme we were able to produce and prepare <SMALL>D</SMALL>&#8208;glucose&#8208;6&#8208;phosphate, <I>N</I>&#8208;acetyl&#8208;<SMALL>D</SMALL>&#8208;glucosamine&#8208;6&#8208;phosphate, allyl phosphate, dihydroxyacetone phosphate, glycerol&#8208;1&#8208;phosphate, and inosine&#8208;5&prime;&#8208;monophosphate from the corresponding primary alcohol on gram scale using either a fed&#8208;batch reactor or a continuous&#8208;flow packed&#8208;bed reactor.</P>

발행연도

2012

ISSN

0947-6539

ISSN

1521-3765

18

21

페이지

pp.6604-6609

주제어

biocatalysis; green chemistry; immobilization; microreactors; phosphorylation

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논문; 2012-12-31

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