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Glycerol and mixture of carbon sources conversion to hydrogen by Clostridium beijerinckii DSM791 and effects of various heavy metals on hydrogenase activity

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논문

Glycerol and mixture of carbon sources conversion to hydrogen by Clostridium beijerinckii DSM791 and effects of various heavy metals on hydrogenase activity

학술지

International journal of hydrogen energy

저자명

Trchounian, Karen; Mü ller, Nicolai; Schink, Bernhard; Trchounian, Armen

초록

<P><B>Abstract</B></P> <P>Hydrogen is a carbon-neutral energy feedstock which is produced during fermentation of various carbon sources. The genomes of clostridia encode mainly [Fe-Fe]-hydrogenases. <I>Clostridium beijerinckii</I> DSM791 performed anaerobic fermentation of glycerol in batch culture at pH 7.5 and pH 5.5 and produced H<SUB>2</SUB>. At pH 7.5, the glycerol consumption rate was 3.7 g/g cell mass/h, which was higher than that at pH 5.5. H<SUB>2</SUB> production reached 5 mmol/h/g cell mass at pH 7.5. The specific hydrogenase activity was &sim;1.4 fold higher if cells were grown on glycerol compared to cells grown on glucose. Single (Fe<SUP>2+</SUP>, Fe<SUP>3+</SUP>, Ni<SUP>2+</SUP>) or mixed supply of metals (Fe<SUP>2+</SUP> and Ni<SUP>2+</SUP>) increased the specific hydrogenase activity by &sim;50%. These results suggest that <I>C. beijerinckii</I> DSM791 could be used as a potential H<SUB>2</SUB> producer. It may help to further enhance H<SUB>2</SUB> production using different industrial or agricultural wastes where glycerol and other carbon sources are present.</P> <P><B>Highlights</B></P> <P> <UL> <LI> <I>Clostridium beijerinckii</I> DSM791 converted glycerol to H<SUB>2</SUB> at pH 7.5 and pH 5.5. </LI> <LI> At pH 7.5, the glycerol consumption rate was 3.7 g/g cell matter/h and it was higher than at pH 5.5. </LI> <LI> H<SUB>2</SUB> production reached 5 mmol/h/g cell mass at pH 7.5. </LI> <LI> Hyd activity was &sim;1.4 fold higher if cells were grown on glycerol compared to cells grown on glucose. </LI> <LI> Fe<SUP>2+</SUP>, Fe<SUP>3+</SUP>, Ni<SUP>2+</SUP> or mixed supply of metals (Fe<SUP>2+</SUP> and Ni<SUP>2+</SUP>) increased the Hyd activity by &sim;50%. </LI> </UL> </P>

발행연도

2017

발행기관

Elsevier

ISSN

0360-3199

ISSN

1879-3487

42

12

페이지

pp.7875-7882

주제어

Fermentation; Hydrogen production; Glycerol and mixed carbon substrates; pH; Hydrogenases; Clostridium beijerinckii

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논문; 2017-03-01

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