Search

Development of a GIN11/FRT-based multiple-gene integration technique affording inhibitor-tolerant, hemicellulolytic, xylose-utilizing abilities to industrial Saccharomyces cerevisiae strains for ethanol production from undetoxified lignocellulosic hemicelluloses

메타 데이터

바이오화학분류
    • 바이오플라스틱
      1. 플라스틱
    • 바이오정밀화학
      1. 용매
      2. 화학제품
      3. 연료
    • 화장품용 기능성소재
      1. 계면활성제⁄증점제
    • 의료용 화학소재
      1. 식품첨가제
논문

Development of a GIN11/FRT-based multiple-gene integration technique affording inhibitor-tolerant, hemicellulolytic, xylose-utilizing abilities to industrial Saccharomyces cerevisiae strains for ethanol production from undetoxified lignocellulosic hemicelluloses

학술지

Microbial cell factories

저자명

Hasunuma, Tomohisa; Hori, Yoshimi; Sakamoto, Takatoshi; Ochiai, Misa; Hatanaka, Haruyo; Kondo, Akihiko

초록

<P><B>Background</B></P><P>Bioethanol produced by the yeast <I>Saccharomyces cerevisiae</I> is currently one of the most promising alternatives to conventional transport fuels. Lignocellulosic hemicelluloses obtained after hydrothermal pretreatment are important feedstock for bioethanol production. However, hemicellulosic materials cannot be directly fermented by yeast: xylan backbone of hemicelluloses must first be hydrolyzed by heterologous hemicellulases to release xylose, and the yeast must then ferment xylose in the presence of fermentation inhibitors generated during the pretreatment.</P><P><B>Results</B></P><P>A GIN11/FRT-based multiple-gene integration system was developed for introducing multiple functions into the recombinant <I>S. cerevisiae</I> strains engineered with the xylose metabolic pathway. Antibiotic markers were efficiently recycled by a novel counter selection strategy using galactose-induced expression of both FLP recombinase gene and <I>GIN11</I> flanked by FLP recombinase recognition target (FRT) sequences. Nine genes were functionally expressed in an industrial diploid strain of <I>S. cerevisiae</I>: endoxylanase gene from <I>Trichoderma reesei</I>, xylosidase gene from <I>Aspergillus oryzae</I>, &beta;-glucosidase gene from <I>Aspergillus aculeatus</I>, xylose reductase and xylitol dehydrogenase genes from <I>Scheffersomyces stipitis</I>, and <I>XKS1</I>, <I>TAL1</I>, <I>FDH1</I> and <I>ADH1</I> variant from <I>S. cerevisiae.</I> The genes were introduced using the homozygous integration system and afforded hemicellulolytic, xylose-assimilating and inhibitor-tolerant abilities to the strain. The engineered yeast strain demonstrated 2.7-fold higher ethanol titer from hemicellulosic material than a xylose-assimilating yeast strain. Furthermore, hemicellulolytic enzymes displayed on the yeast cell surface hydrolyzed hemicelluloses that were not hydrolyzed by a commercial enzyme, leading to increased sugar utilization for improved ethanol production.</P><P><B>Conclusions</B></P><P>The multifunctional yeast strain, developed using a GIN11/FRT-based marker recycling system, achieved direct conversion of hemicellulosic biomass to ethanol without the addition of exogenous hemicellulolytic enzymes. No detoxification processes were required. The multiple-gene integration technique is a powerful approach for introducing and improving the biomass fermentation ability of industrial diploid <I>S. cerevisiae</I> strains.</P><P><B>Electronic supplementary material</B></P><P>The online version of this article (doi:10.1186/s12934-014-0145-9) contains supplementary material, which is available to authorized users.</P>

발행연도

2014

발행기관

BioMed Central

라이선스

cc-by

ISSN

1475-2859

13

페이지

pp.145

주제어

Bioethanol; Cell surface display; Inhibitor tolerance; Lignocellulose; Maker recycling; Saccharomyces cerevisiae

0건의 논문이 있습니다.

0건의 특허가 있습니다.

0건의 무역이 있습니다.

1건의 후보군 물질이 있습니다.

1 2023-12-11

논문; 2014-01-01

Export

About

Search

Trend