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A biocatalytic cascade for the conversion of fatty acids to fatty amines

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논문

A biocatalytic cascade for the conversion of fatty acids to fatty amines

학술지

Green chemistry : an international journal and green chemistry resource : GC

저자명

Citoler, Joan; Derrington, Sasha R.; Galman, James L.; Bevinakatti, Han; Turner, Nicholas J.

초록

<P>Fatty amine synthesis from renewable sources is an energetically-demanding process involving toxic metal catalysts and harsh reaction conditions as well as selectivity problems. Herein we present a mild, biocatalytic alternative to the conventional amination of fatty acids through a one-pot tandem cascade performed by a carboxylic acid reductase (CAR) and a transaminase (&omega;-TA). Saturated and unsaturated fatty acids, with carbon chain lengths ranging from C<SUB>6</SUB> to C<SUB>18</SUB>, were successfully aminated obtaining conversions of up to 96%.</P><P>Graphic Abstract</P><P>A mild, biocatalytic alternative to the conventional amination of fatty acids through a one-pot tandem cascade performed by a carboxylic acid reductase (CAR) and a transaminase (&omega;-TA).<BR/><IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c9gc02260k'/><BR/></P>

발행연도

2019

발행기관

The Royal Society of Chemistry

ISSN

1463-9262

ISSN

1463-9270

21

18

페이지

pp.4932-4935

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논문; 2019-01-01

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