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Chemo-enzymatic Baeyer-Villiger oxidation of 4-methylcyclohexanone via kinetic resolution of racemic carboxylic acids: direct access to enantioenriched lactone

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논문

Chemo-enzymatic Baeyer-Villiger oxidation of 4-methylcyclohexanone via kinetic resolution of racemic carboxylic acids: direct access to enantioenriched lactone

학술지

Chemical communications : Chem comm

저자명

Droż dż , Agnieszka; Chrobok, Anna

초록

<P>A new method for the asymmetric chemo-enzymatic Baeyer&ndash;Villiger oxidation of prochiral 4-methylcyclohexanone to (<I>R</I>)-4-methylcaprolactone in the presence of (&plusmn;)-4-methyloctanoic acid, <I>Candida Antarctica</I> lipase B and 30% aq. H<SUB>2</SUB>O<SUB>2</SUB> has been developed. A mechanism for the asymmetric induction based on kinetic resolution of racemic carboxylic acids is proposed.</P><BR><BR><P>Graphic Abstract</P><P>A new method for the asymmetric chemo-enzymatic Baeyer&ndash;Villiger oxidation of 4-methylcyclohexanone to enantioenriched lactone in the presence of (&plusmn;)-4-methyloctanoic acid, <I>Candida Antarctica</I> lipase B and 30% aq. H<SUB>2</SUB>O<SUB>2</SUB> has been developed.<BR><IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c5cc08519e'><BR></P>

발행연도

2016

발행기관

The Royal Society of Chemistry

ISSN

1359-7345

ISSN

1364-548x

52

6

페이지

pp.1230-1233

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1 2023-12-11

논문; 2016-12-31

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