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Urease-catalyzed synthesis of aminocyanopyridines from urea under fully green conditions

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논문

Urease-catalyzed synthesis of aminocyanopyridines from urea under fully green conditions

학술지

Journal of molecular catalysis. B, Enzymatic

저자명

Tamaddon, F.; Ghazi, S.; Noorbala, M.R.

초록

This is an original work on catalytic performance of urease in organic synthesis which in one-pot dissociation of urea and condensation of the in situ generated ammonia with aldehydes, acetophenones, and malononitrile occurs in water to give 2-amino-3-cyanopyridines. Comparative experiments with ammonium salts supported the enzymatic specify of 0.01g/mL (50U/mg) of urease for bio-production of ammonia, while trace amount of heavy metal ions such as Pb<SUP>2+</SUP>, Hg<SUP>2+</SUP>, and Ag<SUP>+</SUP> inhibit these specific reactions. The scalability and promiscuity of urease facilitate the applicability of the process for biotechnological organic reactions based on ammonia.

발행연도

2016

발행기관

Elsevier

ISSN

1381-1177

ISSN

1873-3158

127

페이지

pp.89-92

주제어

Urease; Enzymatic reactions; In situ generation of ammonia; Biocompatible; Pyridines

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1 2023-12-11

논문; 2016-05-01

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