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Overexpression and characterization of a glucose-tolerant β-glucosidase from Thermotoga thermarum DSM 5069T with high catalytic efficiency of ginsenoside Rb1 to Rd

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논문

Overexpression and characterization of a glucose-tolerant β-glucosidase from Thermotoga thermarum DSM 5069T with high catalytic efficiency of ginsenoside Rb1 to Rd

학술지

Journal of molecular catalysis. B, Enzymatic

저자명

Zhao, L.; Xie, J.; Zhang, X.; Cao, F.; Pei, J.

초록

The &beta;-glucosidase gene Tt-bgl from Thermotoga thermarum DSM 5069T was cloned and overexpressed in Escherichia coli. A simple strategy, induction at 37<SUP>o</SUP>C with no IPTG, was explored to reduce the inclusion bodies, by which the activity of Tt-BGL was 13U/mL in LB medium. Recombinant Tt-BGL was purified by heat treatment followed by Ni-NTA affinity. The optimal activity was at pH 4.8 and 90<SUP>o</SUP>C. The activity of Tt-BGL was significantly enhanced by methanol and Al<SUP>3+</SUP>. The enzyme was stable over pH range of 4.4-8.0, and had a 2-h half life at 90<SUP>o</SUP>C. The V<SUB>max</SUB> for p-nitrophenyl-&beta;-d-glucopyranoside and ginsenoside Rb1 was 142U/mg and 107U/mg, while the K<SUB>m</SUB> was 0.59mM and 0.15mM, respectively. The activity of the enzyme was not inhibited by ginsenoside Rb1 (36g/L). It was activated by glucose at concentrations lower that 400mM. With glucose further increasing, the activity of Tt-BGL was gradually inhibited, but remained 50% of the original value in even as high as 1500mM glucose. Under the optimal conditions, Tt-BGL transformed ginsenoside Rb1 (36g/L) to Rd by 95% in 1h.

발행연도

2013

발행기관

Elsevier

ISSN

1381-1177

ISSN

1873-3158

95

페이지

pp.62-69

주제어

Overexpression; Glucose-tolerant β-glucosidase; Thermotoga thermarum; Biotransformation; Ginsenoside

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1 2023-12-11

논문; 2013-11-01

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