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Optimization of the yield of dark microaerobic production of hydrogen from lactate by Rhodopseudomonas palustris

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논문

Optimization of the yield of dark microaerobic production of hydrogen from lactate by Rhodopseudomonas palustris

학술지

Bioresource technology : biomass, bioenergy, biowastes, conversion technologies, biotransformations, production technologies

저자명

Lazaro, Carolina Zampol; Hitit, Zeynep Yilmazer; Hallenbeck, Patrick C.

초록

<P><B>Abstract</B></P> <P>Hydrogen yields of dark fermentation are limited due to the need to also produce reduced side products, and photofermentation, an alternative, is limited by the need for light. A relatively new strategy, dark microaerobic fermentation, could potentially overcome both these constraints. Here, application of this strategy demonstrated for the first time significant hydrogen production from lactate by a single organism in the dark. Response surface methodology (RSM) was used to optimize substrate and oxygen concentration as well as inoculum using both (1) regular batch and (2) O<SUB>2</SUB> fed batch cultures. The highest hydrogen yield (HY) was observed under regular batch (1.4&plusmn;0.1molH<SUB>2</SUB>/mollactate) and the highest hydrogen production (HP) (173.5&micro;molH<SUB>2</SUB>) was achieved using O<SUB>2</SUB> fed batch. This study has provided proof of principal for the ability of microaerobic fermentation to drive thermodynamically difficult reactions, such as the conversion of lactate to hydrogen.</P> <P><B>Highlights</B></P> <P> <UL> <LI> High hydrogen yield from lactate under dark microaerobic conditions demonstrated. </LI> <LI> Addition of fixed nitrogen had a negative effect on hydrogen production. </LI> <LI> HY was higher using regular batch culture, HP was higher using O<SUB>2</SUB> fed batch. </LI> <LI> Agitation plays an important role in MADF by augmenting oxygen diffusion. </LI> </UL> </P>

발행연도

2017

발행기관

Elsevier

라이선스

publisher-specific-oa

ISSN

0960-8524

245

1

페이지

pp.123-131

주제어

Photosynthetic bacterium; Dark hydrogen production; Lactate to hydrogen; Microaerobic fermentation; Fed batch; RSM

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1 2023-12-11

논문; 2017-12-01

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