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Seven-enzyme in vitro cascade to (3R)-3-hydroxybutyryl-CoA

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논문

Seven-enzyme in vitro cascade to (3R)-3-hydroxybutyryl-CoA

학술지

Organic & biomolecular chemistry

저자명

Valencia, Luis E.; Zhang, Zhicheng; Cepeda, Alexis J.; Keatinge-Clay, Adrian T.

초록

<P>Economical and environmentally-friendly routes to convert feedstock chemicals like acetate into valuable chiral products such as (<I>R</I>)-3-hydroxybutyrate are in demand. Here, seven enzymes (CoaA, CoaD, CoaE, ACS, BktB, PhaB, and GDH) are employed in a one-pot, <I>in vitro</I>, biocatalytic synthesis of (3<I>R</I>)-3-hydroxybutyryl-CoA, which was readily isolated. This platform generates not only chiral diketide building blocks but also desirable CoA derivatives.</P><P>Graphic Abstract</P><P>Economical and environmentally-friendly routes to convert feedstock chemicals like acetate into valuable chiral products such as (<I>R</I>)-3-hydroxybutyrate are in demand.<BR/><IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c8ob02858c'/><BR/></P>

발행연도

2019

발행기관

The Royal Society of Chemistry

ISSN

1477-0520

ISSN

1477-0539

17

6

페이지

pp.1375-1378

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1 2023-12-11

논문; 2019-12-31

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