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Salting-out of 1,3-propanediol from aqueous solutions by inorganic electrolytes

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논문

Salting-out of 1,3-propanediol from aqueous solutions by inorganic electrolytes

학술지

Journal of chemical technology and biotechnology

저자명

Xie, Shaoqu; Qiu, Xueqing; Ji, Weini; Yi, Conghua

초록

<P><B>ABSTRACT</B></P><P><B>BACKGROUND</B></P><P>The cost of 1,3&#8208;propanediol (1,3&#8208;PD) microbial production depends very much on the separation of 1,3&#8208;PD from the fermentation broth. This work develops a salting&#8208;out process separating 1,3&#8208;PD from aqueous solutions. The salting&#8208;out effects of K<SUB>2</SUB>CO<SUB>3</SUB>, K<SUB>3</SUB>PO<SUB>4</SUB>, and K<SUB>4</SUB>P<SUB>2</SUB>O<SUB>7</SUB> on the liquid&ndash;liquid phase equilibria for different aqueous solutions of 1,3&#8208;PD were investigated at 298.15 K.</P><P><B>RESULTS</B></P><P>The distribution coefficient and selectivity coefficient of 1,3&#8208;PD increased significantly with increase of the initial salt concentration in the salting&#8208;out systems. Increasing the initial 1,3&#8208;PD concentration in the aqueous solution improved the distribution coefficient and selectivity coefficient of 1,3&#8208;PD, resulting in higher recovery of 1,3&#8208;PD.</P><P><B>CONCLUSION</B></P><P>The solubility of 1,3&#8208;PD in the aqueous phase was mainly determined by the salt species and its concentration. The initial 1,3&#8208;PD concentration in the aqueous solution had a negligible effect on the solubility of 1,3&#8208;PD in the aqueous phase, which showed a linear relation with the molality of salt in the aqueous phase. Moreover, the solubility of 1,3&#8208;PD in the organic phase or the aqueous phase could be predicted by the initial salt concentration. &copy; 2016 Society of Chemical Industry</P>

발행연도

2016

발행기관

John WileySons, Ltd

ISSN

0268-2575

ISSN

1097-4660

91

11

페이지

pp.2793-2801

주제어

salting&#x2010; out; 1, 3&#x2010; propanediol; aqueous solutions; inorganic electrolytes; liquid&#x2013; liquid equilibria; solubility of 1,3&#x2010; PD;

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1 2023-12-11

논문; 2016-02-12

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