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Homolactic acid fermentation by the genetically engineered thermophilic homoacetogen Moorella thermoacetica ATCC 39073

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논문

Homolactic acid fermentation by the genetically engineered thermophilic homoacetogen Moorella thermoacetica ATCC 39073

학술지

Applied and environmental microbiology

저자명

Iwasaki, Yuki; Kita, Akihisa; Yoshida, Koichiro; Tajima, Takahisa; Yano, Shinichi; Shou, Tomohiro; Saito, Masahiro; Kato, Junichi; Murakami, Katsuji; Nakashimada, Yutaka

초록

<P>For the efficient production of target metabolites from carbohydrates, syngas, or H<SUB>2</SUB>-CO<SUB>2</SUB> by genetically engineered <I>Moorella thermoacetica</I>, the control of acetate production (a main metabolite of <I>M. thermoacetica</I>) is desired. Although propanediol utilization protein (PduL) was predicted to be a phosphotransacetylase (PTA) involved in acetate production in <I>M. thermoacetica</I>, this has not been confirmed. Our findings described herein directly demonstrate that two putative PduL proteins, encoded by Moth_0864 (<I>pduL1</I>) and Moth_1181 (<I>pduL2</I>), are involved in acetate formation as PTAs. To disrupt these genes, we replaced each gene with a lactate dehydrogenase gene from <I>Thermoanaerobacter pseudethanolicus</I> ATCC 33223 (<I>T-ldh</I>). The acetate production from fructose as the sole carbon source by the <I>pduL1</I> deletion mutant was not deficient, whereas the disruption of <I>pduL2</I> significantly decreased the acetate yield to approximately one-third that of the wild-type strain. The double-deletion (both <I>pduL</I> genes) mutant did not produce acetate but produced only lactate as the end product from fructose. These results suggest that both <I>pduL</I> genes are associated with acetate formation via acetyl-coenzyme A (acetyl-CoA) and that their disruption enables a shift in the homoacetic pathway to the genetically synthesized homolactic pathway via pyruvate.</P><P><B>IMPORTANCE</B> This is the first report, to our knowledge, on the experimental identification of PTA genes in <I>M. thermoacetica</I> and the shift of the native homoacetic pathway to the genetically synthesized homolactic pathway by their disruption on a sugar platform.</P>

발행연도

2017

발행기관

American Society for Microbiology

ISSN

0099-2240

ISSN

1098-5336

83

8

페이지

pp.e00247-17-e00247-17

주제어

thermophilic; acetogen; Moorella; transformation; biomass; sugar; syngas; fermentation

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1 2023-12-11
2 2023-12-11

논문; 2017-04-15

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