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Utilization of excess NADH in 2,3-butanediol-deficient Klebsiella pneumoniae for 1,3-propanediol production

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논문

Utilization of excess NADH in 2,3-butanediol-deficient Klebsiella pneumoniae for 1,3-propanediol production

학술지

Journal of applied microbiology

저자명

Cui, Y.L.; Zhou, J.J.; Gao, L.R.; Zhu, C.Q.; Jiang, X.; Fu, S.L.; Gong, H.

초록

<P><B>Abstract</B></P><P><B>Aims</B></P><P>To utilize excess NADH for 1,3&#8208;propanediol production by 2,3&#8208;butanediol&#8208;deficient mutants, the effect of <I>dhaT</I> overexpression in two distinct 2,3&#8208;butanediol&#8208;deficient mutants was investigated.</P><P><B>Methods and Results</B></P><P>Two 2,3&#8208;butanediol&#8208;deficient mutants, KG1&#8208;3 (blocking of the 2,3&#8208;butanediol pathway only) and KG1&#8208;5 (blocking of both of 2,3&#8208;butanediol and lactate pathways) were constructed. Our results showed that although the intracellular redox balance (NADH/NAD<SUP>+</SUP>) was extremely high at the end of fermentation for both mutants, the status of intracellular redox in KG1&#8208;5 was maintained at a normal level following the first stage of fermentation. Analysis of cell growth and metabolite formation confirmed the inhibition of excess lactate in 2,3&#8208;butanediol pathway&#8208;deficient mutants. Furthermore, <I>dhaT</I> was overexpressed in two 2,3&#8208;butanediol&#8208;deficient mutants (KG1&#8208;3T and KG1&#8208;5T). In KG1&#8208;5T, the intracellular redox balance was restored to normal and 1,3&#8208;propanediol production increased. The yield of 1,3&#8208;propanediol from glycerol in KG1&#8208;5T was also restored to a normal level of 0&middot;6.</P><P><B>Conclusions</B></P><P>The excess NADH in both the 2,3&#8208;butanediol&#8208; and lactate&#8208;deficient mutants can be used by overexpresstion of <I>dhaT</I>.</P><P><B>Significance and Impact of Study</B></P><P>The metabolic flux tended to increase lactate production by the abolishment of the 2,3&#8208;butanediol pathway in <I>Klebsiella pneumoniae,</I> and the high accumulation of lactate prevented the cell from using excess NADH, thereby inhibiting cell growth and 1,3&#8208;propanediol production.</P>

발행연도

2014

ISSN

1364-5072

ISSN

1365-2672

117

3

페이지

pp.690-698

주제어

1,3&#x2010; propanediol; 2,3&#x2010; butanediol; dhaT overexpression; Klebsiella pneumoniae; lactate; NADH;

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논문; 2014-12-31

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