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Biological hydrogen production by Anabaena sp. - Yield, energy and CO2 analysis including fermentative biomass recovery

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논문

Biological hydrogen production by Anabaena sp. - Yield, energy and CO2 analysis including fermentative biomass recovery

학술지

International journal of hydrogen energy

저자명

Ferreira, Ana F.; Marques, Ana C.; Batista, Ana P.; Marques, Paula A.S.S.; Gouveia, Luí sa; Silva, Carla M.

초록

<P><B>Abstract</B></P><P>This paper presents laboratory results of biological production of hydrogen by photoautrotophic cyanobacterium <I>Anabaena</I> sp. Additional hydrogen production from residual <I>Cyanobacteria</I> fermentation was achieved by <I>Enterobacter aerogenes</I> bacteria. The authors evaluated the yield of H<SUB>2</SUB> production, the energy consumption and CO<SUB>2</SUB> emissions and the technological bottlenecks and possible improvements of the whole energy and CO<SUB>2</SUB> emission chain.</P><P>The authors did not attempt to extrapolate the results to an industrial scale, but to highlight the processes that need further optimization.</P><P>The experiments showed that the production of hydrogen from cyanobacteria <I>Anabaena</I> sp. is technically viable. The hydrogen yield for this case was 0.0114&nbsp;kg<SUB>H2</SUB>/kg<SUB>biomass</SUB> which had a rough energy consumption of 1538&nbsp;MJ/MJ<SUB>H2</SUB> and produced 114640&nbsp;gCO<SUB>2</SUB>/MJ<SUB>H2</SUB>. The use of phototrophic residual cyanobacteria as a substrate in a dark-fermentation process increased the hydrogen yield by 8.1% but consumed 12.0% more of energy and produced 12.1% more of CO<SUB>2</SUB> showing that although the process increased the overall efficiency of hydrogen production it was not a viable energy and CO<SUB>2</SUB> emission solution. To make cyanobacteria-based biofuel production energy and environmentally relevant, efforts should be made to improve the hydrogen yield to values which are more competitive with glucose yields (0.1&nbsp;kg<SUB>H2</SUB>/kg<SUB>biomass</SUB>). This could be achieved through the use of electricity with at least 80% of renewables and eliminating the unessential processes (e.g. pre-concentration centrifugation).</P> <P><B>Highlights</B></P><P>&#x025BA; Best H<SUB>2</SUB> photoautotrophic production yield is 0.128 kg<SUB>H2</SUB>/kg<SUB>biomass</SUB> (Ar&nbsp;&plus;&nbsp;CO<SUB>2</SUB>&nbsp;&plus;&nbsp;N<SUB>2</SUB> gas atmosphere; high intensity of light). &#x025BA; Best H<SUB>2</SUB> production, energy and CO<SUB>2</SUB> balance is for Ar&nbsp;&plus;&nbsp;CO<SUB>2</SUB>&nbsp;&plus;&nbsp;20% N<SUB>2</SUB> gas atmosphere and medium light intensity. &#x025BA; H<SUB>2</SUB> yield can be increased 8% using the biomass leftovers but with 12% energy and CO<SUB>2</SUB> increase. &#x025BA; Improving H<SUB>2</SUB> yield and using high shares of renewable electricity, allows significant decrease of energy and CO<SUB>2</SUB>. &#x025BA; Cyanobacteria-based production of H2 must be further investigated to be sustainable relevant.</P>

발행연도

2012

발행기관

Elsevier

ISSN

0360-3199

ISSN

1879-3487

37

1

페이지

pp.179-190

주제어

Cyanobacteria; Biohydrogen; Photoautotrophic production; Energy balance; CO2 emissions

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논문; 2012-12-31

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