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Metabolic engineering and adaptive evolution of Escherichia coli KO11 for ethanol production through the Entner-Doudoroff and the pentose phosphate pathways

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논문

Metabolic engineering and adaptive evolution of Escherichia coli KO11 for ethanol production through the Entner-Doudoroff and the pentose phosphate pathways

학술지

Journal of chemical technology and biotechnology

저자명

Huerta‐ Beristain, Gerardo; Cabrera‐ Ruiz, Rosina; Hernandez‐ Chavez, Georgina; Bolivar, Francisco; Gosset, Guillermo; Martinez, Alfredo

초록

<P><B>Abstract</B></P><P><B>BACKGROUND</B></P><P>Ethanologenic <I>Escherichia coli</I> KO11 was modified to channel carbon flux from glucose through the Entner&ndash;Doudoroff (ED&#8208;P) and pentose phosphate (PP&#8208;P) pathways by using a phosphoglucose isomerase (<I>pgi</I>) knockout in the glycolytic pathway. This strain grows very slowly under non&#8208;aerated conditions with minimal media supplemented with 4% glucose. To improve the capacity to grow, KO11 &Delta;<I>pgi</I> was evolved for 60 days; the resultant strain was named KO11 E35, which directs the carbon flux through the PP&#8208;P and ED&#8208;P to lactate and acetate production.</P><P><B>RESULTS</B></P><P>The activities of glucose&#8208;6&#8208;phosphate dehydrogenase and the ED&#8208;P enzymes increased 17&#8208;fold and 2&#8208;fold, respectively, in KO11 E35 in comparison with KO11. A homoethanologenic derivative was constructed from KO11 E35 by deleting the <I>pta</I>, <I>ack</I> and <I>ldh</I> genes, yielding the KO11 PPAL strain. This strain channels most of the carbon flux from pyruvate to ethanol and increased expression of heterologous pyruvate decarboxylase and alcohol dehydrogenase from <I>Zymomonas mobilis</I> allowed us to obtain specific ethanol production rates similar to those found in KO11, but with half the cell mass, i.e. larger ethanol/glucose and ethanol/biomass yields.</P><P><B>CONCLUSIONS</B></P><P>These results suggest that it is possible to obtain the same carbon flux using the PP&#8208;P and ED&#8208;P as when using the Embden&ndash;Meyerhof&ndash;Parnas pathway for glucose catabolism to ethanol. &copy; 2016 Society of Chemical Industry</P>

발행연도

2017

발행기관

John WileySons, Ltd

ISSN

0268-2575

ISSN

1097-4660

92

5

페이지

pp.990-996

주제어

ethanologenic Escherichia coli; glucose; ethanol; pentose phosphate pathway; Entner&#x2013; Doudoroff pathway; adaptive evolution;

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논문; 2017-12-31

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