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Comparison of Three Thermostable β-Glucosidases for Application in the Hydrolysis of Soybean Isoflavone Glycosides

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논문

Comparison of Three Thermostable β-Glucosidases for Application in the Hydrolysis of Soybean Isoflavone Glycosides

학술지

Journal of agricultural and food chemistry

저자명

Song, Xiangfei; Xue, Yemin; Wang, Qilei; Wu, Xixi

초록

<P>A novel thermostable &beta;-glucosidase (Te-BglA) from <I>Thermoanaerobacter ethanolicus</I> JW200 was cloned, characterized and compared for its activity against isoflavone glycosides with two &beta;-glucosidases (Tm-BglA, Tm-BglB) from <I>Thermotoga maritima</I>. Te-BglA exhibited maximum hydrolytic activity toward <I>p</I>NP-&beta;-<SMALL>d</SMALL>-glucopyranoside (<I>p</I>NPG) at 80 &deg;C and pH 7.0, was stable for a pH range of 4.6&minus;7.8 and at 65 &deg;C for 3 h, and had the lowest <I>K</I><SUB>m</SUB> for the natural glycoside salicin and the highest relative substrate specificity (<I>k</I><SUB>cat</SUB>/<I>K</I><SUB>m</SUB>)<SUP>(salicin)</SUP>/(<I>k</I><SUB>cat</SUB>/<I>K</I><SUB>m</SUB>)<SUP>(<I>p</I>NPG)</SUP> among the three enzymes. It converted isoflavone glycosides, including malonyl glycosides, in soybean flour to their aglycons more efficiently than Tm-BglA and Tm-BglB. After 3 h of incubation at 65 &deg;C, Te-BglA produced complete hydrolysis of four isoflavone glycosides (namely, daidzin, genistin and their malonylated forms), exhibiting higher productivity of genistein and daidzein than the other two &beta;-glucosidases. Our results suggest that Te-BglA is preferable to Tm-BglA and Tm-BglB, but all three enzymes have great potential applications in converting isoflavone glycosides into their aglycons.</P>

발행연도

2011

발행기관

American Chemical Society

ISSN

0021-8561

ISSN

1520-5118

59

5

페이지

pp.1954-1961

주제어

thermostable β-glucosidase; hydrolysis; soybean flour; isoflavone glycosides

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1 2023-12-11

논문; 2011-02-02

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