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Photocatalytic degradation of lignin on synthesized Ag-AgCl/ZnO nanorods under solar light and preliminary trials for methane fermentation

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논문

Photocatalytic degradation of lignin on synthesized Ag-AgCl/ZnO nanorods under solar light and preliminary trials for methane fermentation

학술지

Bioresource technology : biomass, bioenergy, biowastes, conversion technologies, biotransformations, production technologies

저자명

Li, H.; Lei, Z.; Liu, C.; Zhang, Z.; Lu, B.

초록

New photocatalysts, Ag-AgCl/ZnO nanorods, were successfully synthesized in this study by using microwave assisted chemical precipitation and deposition-precipitation-photoreduction methods. The optimal preparation condition was determined as pH 9 in distilled water and 40min for UV light photoreduction of Ag (i.e. Ag<SUB>40</SUB>-AgCl/ZnO) by degradation of methyl orange. This work investigated the feasibility of using Ag<SUB>40</SUB>-AgCl/ZnO to degrade lignin under natural solar light and then subsequent methane production with influencing factors like solution pH, dosage of catalyst and initial lignin concentration being considered. <SUP>?</SUP>OH radicals were found to play the most important role in the photocatalytic process, and the new prepared catalyst possessed stable photocatalytic activity after 7 cycles' utilization. During the subsequent biogasification, the degraded lignin obtained from 120min photocatalysis yielded 184ml methane and 325ml biogas for per gram of removed total organic carbon, increased by 10.9% and 23.1%, respectively compared to the control.

발행연도

2015

발행기관

Elsevier Applied Science

ISSN

0960-8524

175

페이지

pp.494-501

주제어

Ag-AgCl/ZnO nanorods; Lignin; Photocatalysis; Methane production

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1 2023-12-11

논문; 2015-12-31

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