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Enzymatic synthesis of halogen derivatives of L-phenylalanine and phenylpyruvic acid stereoselectively labeled with hydrogen isotopes in the side chain

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논문

Enzymatic synthesis of halogen derivatives of L-phenylalanine and phenylpyruvic acid stereoselectively labeled with hydrogen isotopes in the side chain

학술지

Journal of labelled compounds & radiopharmaceuticals

저자명

Pałka, Katarzyna; Podsadni, Katarzyna; Pają k, Małgorzata

초록

<P>Halogenated, labeled with deuterium, tritium or doubly labeled with deuterium and tritium in the 3<I>S</I> position of the side chain isotopomers of L&#x2010;phenylalanine and phenylpyruvic acid were synthesized. Isotopomers of halogenated L&#x2010;phenylalanine were obtained by addition of ammonia from isotopically enriched buffer solution to the halogenated derivative of (<I>E</I>)&#x2010;cinnamic acid catalyzed by phenylalanine ammonia lyase. Isotopomers of halogenated phenylpyruvic acid were obtained enzymatically by conversion of the appropriate isotopomer of halogenated L&#x2010;phenylalanine in the presence of phenylalanine dehydrogenase. As a source of deuterium was used deuterated water, as a source of tritium was used a solution of highly diluted tritiated water. The labeling takes place in good yields and with high deuterium atom% abundance.</P>

발행연도

2023

발행기관

Wiley (John WileySons)

ISSN

0362-4803

ISSN

1099-1344

66

11

페이지

pp.362-368

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1 2023-12-11

논문; 2023-09-01

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