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Production and characterization of cellulolytic enzyme from Penicillium oxalicum GZ-2 and its application in lignocellulose saccharification

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논문

Production and characterization of cellulolytic enzyme from Penicillium oxalicum GZ-2 and its application in lignocellulose saccharification

학술지

Biomass & bioenergy

저자명

Liao, Hanpeng; Fan, XiaoTeng; Mei, Xinlan; Wei, Zhong; Raza, Waseem; Shen, Qirong; Xu, Yangchun

초록

<P><B>Abstract</B></P> <P>A large amount of FPase (1.4U/mL), CMCase (2.0U/mL), cellobiohydrolase (0.6U/mL), and &beta;-glucosidase (2.7U/mL) activities were produced when <I>Penicillium oxalicum</I> GZ-2 was grown on rice straw in a 5 L bioreactor. The zymography demonstrated that the expression abundance of cellulose-degrading proteins (35&ndash;70 kDa) responded to high cellulolytic enzymes activity. Cellobiohydrolase, exo-beta-1,3-glucanase, endo-beta-1,4-glucanase, swollenin, and other glycoside hydrolases were identified in visible hydrolyzed bands in zymogram gel using MALDI-TOF-MS/MS. The relative proportions of cellulose-degrading proteins were 50.0%, 45.7%, and 44.1% in the crude enzymes induced by wheat straw, rice straw, and corn stover, respectively. It suggested that the majority of extracellular proteins were cellulose-degrading enzymes induced by agricultural wastes. The optimized pH and temperature for CMCase and &beta;-glucosidase activity were 3.0 at 50 &deg;C and 5.0 at 60 &deg;C, respectively. The CMCase and &beta;-glucosidase showed remarkable stability at pH 4.0&ndash;9.0 and 3.0&ndash;7.0 with 80% of the maximum activity, respectively. Although the FPase activity was similar, the &beta;-glucosidase activity of <I>P. oxalicum</I> GZ-2 was 2.8 times greater than that of <I>Trichoderma reesei</I> RUT-C30. The culture supernatants of <I>P. oxalicum</I> GZ-2 showed more efficiently capability to enzymatic hydrolysis of Avicel and corncob compared to commercial cellulase. For the saccharification of alkali-pretreated corncob, a higher reducing sugar and glucose yield was obtained using the culture supernatants from <I>P. oxalicum</I> GZ-2 than those from <I>T. reesei</I> RUT-C30. However, the highest sugar yields obtained from the mixture of enzymes indicated that a better design cocktail was also important for hydrolyzing biomass.</P> <P><B>Graphical abstract</B></P> <P>[DISPLAY OMISSION]</P>

발행연도

2015

발행기관

Elsevier

ISSN

0961-9534

74

페이지

pp.122-134

주제어

Penicillium oxalicum; Cellulolytic enzymes; Culture supernatant; Agricultural wastes; Saccharification

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논문; 2015-03-01

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